There are a few apps on the Mac App Store that let you map controller presses as keyboard keys.
this post was submitted on 18 Jun 2023
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Macintosh Gamers ๐ฅ๏ธ๐ | Gaming on macOS and Mac hardware
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Pressing the ps button opens the mac's launchpad on your end? It did that in mine, and I could select and run apps with arrows+x. But I don't know if chrome supports joystick controls. Maybe try steam big picture mode? I think it has a web browser in it.